Unusual Features of Depletion Interactions in Soft Polymer-Based Colloids Mixed with Linear Homopolymers

Author(s)
Manuel Camargo, Christos Likos
Abstract

We investigate the influence of the addition of polymer chains on the effective interaction between star polymers, as a model for the depletion potential in ultrasoft mixtures. The effects of size ratio and chain polymer concentration on the chain-modified star-star interactions at good (athermal) solvent conditions are investigated. For both hard sphere mixtures and colloid-nonadsorbing polymer mixtures the range of the depletion interaction increases with the size ratio. For the systems at hand, the range of the depletion potential is insensitive to the size of the depletant polymer. The physical origin of this and the associated effects, as well as a mapping of the mixtures onto a one-component system, are discusssed.

Organisation(s)
Computational and Soft Matter Physics
External organisation(s)
Heinrich-Heine-Universität Düsseldorf
Journal
Physical Review Letters
Volume
104
No. of pages
4
ISSN
0031-9007
DOI
https://doi.org/10.1103/PhysRevLett.104.078301
Publication date
2010
Peer reviewed
Yes
Austrian Fields of Science 2012
1030 Physics, Astronomy
Portal url
https://ucrisportal.univie.ac.at/en/publications/d2517897-5437-433d-8909-ae9884e83e25