Interfacial and wetting behaviour of phase-separating ultrasoft mixtures

Author(s)
Manuel Camargo, Christos Likos
Abstract

We apply density functional theory to study the interfacial properties of a phase-separating binary fluid of ultrasoft particles, whose interaction potentials belong to the family of the so-called generalized exponential models (GEM). By using the formalism of the density functional theory within the mean-field approximation, we investigate the equilibrium density profiles for each component at the free interface as well as at a repulsive, flat wall. We show that the studied system can lead to first-order wetting transition which is characterized by a layering-like behaviour due to the clustering properties of GEM particles.

Organisation(s)
Computational and Soft Matter Physics
External organisation(s)
Heinrich-Heine-Universität Düsseldorf
Journal
Molecular Physics: an international journal in the field of chemical physics
Volume
109
Pages
1121-1132
No. of pages
12
ISSN
0026-8976
DOI
https://doi.org/10.1080/00268976.2010.548344
Publication date
2011
Peer reviewed
Yes
Austrian Fields of Science 2012
103036 Theoretical physics, 103015 Condensed matter, 103029 Statistical physics
Portal url
https://ucrisportal.univie.ac.at/en/publications/396b41f3-48c1-4f2f-8127-3a2544e450e2