Anomalous relaxation of coarsening foams with viscoelastic continuous phases

Author(s)
Chiara Guidolin, Emmanuelle Rio, Roberto Cerbino, Anniina Salonen, Fabio Giavazzi
Abstract

We investigate the ultraslow structural relaxation of ageing foams with rheologically tunable continuous phases. We probe the bubble dynamics associated with pressure-driven foam coarsening using differential dynamic microscopy, which allows characterising the sample dynamics in reciprocal space with imaging experiments. Similar to other out-of-equilibrium jammed soft systems, these foams exhibit compressed exponential relaxations, with a ballistic-like linear dependency of the relaxation rate on the scattering wavevector. By tuning the rheology of the continuous phase, we observe changes in the relaxation shape, where stiffer matrices yield larger compression exponents. Our results corroborate recent real-space observations obtained using bubble tracking, providing a comprehensive overview of structural relaxation in these complex systems, both in direct and reciprocal space.

Organisation(s)
Computational and Soft Matter Physics
External organisation(s)
Università degli Studi di Milano-Bicocca, Université Paris Saclay
Journal
Soft Matter
Volume
20
Pages
7021-7029
No. of pages
9
ISSN
1744-683X
DOI
https://doi.org/10.1039/D4SM00588K
Publication date
2024
Peer reviewed
Yes
Austrian Fields of Science 2012
103015 Condensed matter, 103045 Light optical microscopy, 103018 Materials physics
Keywords
ASJC Scopus subject areas
Condensed Matter Physics, Chemistry(all)
Portal url
https://ucrisportal.univie.ac.at/en/publications/anomalous-relaxation-of-coarsening-foams-with-viscoelastic-continuous-phases(191c28b9-3f3c-4373-a9f5-decef42ae4bf).html